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Exchange-striction driven ultrafast nonthermal lattice dynamics in NiO

Y. W. Windsor, D. Zahn, R. Kamrla, J. Feldl, H. Seiler, C.-T. Chiang, M. Ramsteiner, W. Widdra, R. Ernstorfer, and L. Rettig – 2021

We use femtosecond electron diffraction to study ultrafast lattice dynamics in the highly correlated antiferromagnetic (AFM) semiconductor NiO. Using the scattering vector (𝘘) dependence of Bragg diffraction, we introduce 𝘘-resolved effective temperatures describing the transient lattice. We identify a nonthermal lattice state with preferential displacement of O compared to Ni ions, which occurs within ∼0.3  ps and persists for 25 ps. We associate this with transient changes to the AFM exchange striction-induced lattice distortion, supported by the observation of a transient 𝘘 asymmetry of Friedel pairs. Our observation highlights the role of spin-lattice coupling in routes towards ultrafast control of spin order.

Title
Exchange-striction driven ultrafast nonthermal lattice dynamics in NiO
Author
Y. W. Windsor, D. Zahn, R. Kamrla, J. Feldl, H. Seiler, C.-T. Chiang, M. Ramsteiner, W. Widdra, R. Ernstorfer, and L. Rettig
Keywords
Antiferromagnetism, Lattice dynamics, Ultrafast magnetic effects, Ultrafast phenomena, Antiferromagnets, Charge-transfer insulators, Electron diffraction
Date
2021
Identifier
DOI: 10.1103/PhysRevLett.126.147202
Appeared in
Phys. Rev. Lett. 126, 147202 (2021)
Type
Text